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Absolute molecular optical Kerr effectspectroscopy of dilute organicsolutions and neat organic liquidsSteven R. Vigil*and Mark G. Kuzyk Department of Physics, Washington State University, Pullman, Washington 99164-2814 Received October 13, 2000; revised manuscript received December 1, 2000We report the results of pump probe optical Kerr effect (OKE) experiments performed on neat solutions ofcarbon tetrachloride, nitrobenzene, methyl methacrylate monomer, binary solutions of the squaraine dye in-dole squarylium, and the phthalocyanine dye silicon phthalocyanine-monomethacrylate, respectively, in car-bon tetrachloride, and solid solutions of indole squarylium and phthalocyanine-monomethacrylate inpoly(methyl methacrylate). Dispersion measurements of the dye solutions were performed in the visible one-photon resonant region of the dyes defined by their linear-absorption spectra. The dyes third-order molecularsusceptibility responsegxxxx(2v2;v1,2v1,v2) in this spectral region is markedly different, withR$gISQ%.
Absolute molecular optical Kerr effect spectroscopy of dilute organic solutions and neat organic liquids Steven R. Vigil* and Mark G. Kuzyk† Department of Physics, Washington State University, Pullman, Washington 99164-2814
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