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Flexible, solid-state, ion-conducting membrane with 3D ...

Flexible, solid-state, ion-conducting membrane with 3 Dgarnet nanofiber networks for lithium batteriesKun (Kelvin) Fua,b,1, Yunhui Gonga,1, Jiaqi Daib, Amy Gonga,b, Xiaogang Hana,b, Yonggang Yaob, Chengwei Wanga,b,Yibo Wangb, Yanan Chenb, Chaoyi Yanb, Yiju Lib, Eric D. Wachsmana,b,2, and Liangbing Hua,b,2aUniversity of Maryland Energy Research Center, University of Maryland, College Park, MD 20742; andbDepartment of Materials Science and Engineering,University of Maryland, College Park, MD 20742 Edited by Yi Cui, Stanford University, Stanford, CA, and accepted by Editorial Board Member Tobin J. Marks May 4, 2016 (received for review January 10,2016)Beyond state-of-the-art lithium-ion battery (LIB) technology withmetallic lithium anodes to replace conventional ion intercalationanode materials is highly desirable because of lithium shighestspecific capacity (3,860 mA/g) and lowest negative electrochem-ical potential ( V vs.)

nanowire fillers, based on perovskite-type lithium-ion–conducting Li 0.33La 0.557TiO 3 material, were shown by Cui and coworkers (22) to enhance the ionic conductivity of the polymer composite elec-

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